Asthana, Saket and Fujiwara, K and Tanaka, K
(2014)
Electrical switching to probe complex phases in a frustrated manganite.
Solid State Communications, 187.
pp. 64-67.
ISSN 0038-1098
Abstract
Electrical switching was used to investigate complex phases induced by Cr-substitution in (Pr1/3Sm2/3)2/3Sr 1/3MnO3. This system was expected to transform from a Type I (Mn4+/Mn3+≈3/7) to Type II (Mn4+/Mn 3+≈1) manganite at critical Cr content, satisfying a virtual Mn4+/Mn3+ ratio close to unity. The phase diagram of (Pr1/3Sm2/3)2/3Sr1/3Mn 0.8Cr0.2O3 including charge/spin ordered/disordered phases was probed by electrical switching. The ferromagnetic insulating phase at <~100 K, located next to the charge-ordered antiferromagnetic phase, exhibited a sudden rise in conductivity upon electric-field biasing. This resulted from the melting of charge ordering, and demonstrated the presence of a crossover regime of two coexisting magnetic orderings.
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